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EnanSET SIGNED

Homogeneous and heterogeneous enantioselective Single Electron Transfer (SET) catalysis in cross-coupling reactions

Total Cost €

EC-Contrib. €

Partnership

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EnanSET project word cloud

Explore the words cloud of the EnanSET project. It provides you a very rough idea of what is the project "EnanSET" about.

absolute consequence relation obtain enanset ti inspired incorporation configuration fragrances extended active pure cross raes provides additionally environmentally electron considerably society esters homogeneous scientific direct activation toxic flavours environmental molecular pharmaceutical enantioselective enantiomerically methodology industry chiral coupling paramount chirality chemical catalysis community structure request compounds heterogeneous pore transfer plays molecules single industrial residues first clean materials mofs titanium reactions green postsynthetic context demand entitled organic complexes redox advantages ni

Project "EnanSET" data sheet

The following table provides information about the project.

Coordinator	UNIVERSIDAD DE GRANADA Organization address address: CUESTA DEL HOSPICIO SN city: GRANADA postcode: 18071 website: www.ugr.es contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.
Coordinator Country	Spain [ES]
Total cost	239˙191 €
EC max contribution	239˙191 € (100%)
Programme	1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
Code Call	H2020-MSCA-IF-2016
Funding Scheme	MSCA-IF-GF
Starting year	2018
Duration (year-month-day)	from 2018-02-01 to 2021-05-01

Partnership

Take a look of project's partnership.

#	participants	country	role	EC contrib. [€]
1	UNIVERSIDAD DE GRANADA UNIVERSIDAD DE GRANADA Organization address address: CUESTA DEL HOSPICIO SN city: GRANADA postcode: 18071 website: www.ugr.es contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.	ES (GRANADA)	coordinator	239˙191.00
2	THE SCRIPPS RESEARCH INSTITUTE THE SCRIPPS RESEARCH INSTITUTE Organization address address: NORTH TORREY PINES ROAD 10550 city: LA JOLLA CA postcode: 9207 website: n.a. contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.	US (LA JOLLA CA)	partner	0.00

Map

Project objective

Chirality of organic molecules plays a paramount role in our society as a consequence of the direct relation between the absolute molecular configuration and many properties and applications of molecular compounds and materials. The demand of enantiomerically pure compounds has increased considerably driven by the request of the pharmaceutical industry, as well as applications such as flavours, fragrances, and materials. In this context, the development of new methodologies to obtain enantiomerically pure compounds has become a challenge for the scientific community. This project entitled “Homogeneous and heterogeneous enantioselective Single Electron Transfer (SET) catalysis in cross-coupling reactions (EnanSET)” aims at developing novel enantioselective SET cross-coupling reactions of redox active esters (RAEs) by Ni-complex due to this kind of compounds do not need previous activation. Moreover, in order to develop more environmentally friendly processes, the methodology will be extended to non-toxic SET complex as titanium complexes, with the goal of developing the first Ti-catalysis of RAEs. Additionally, inspired by demand of the industrial processes, the need to develop clean and green chemical processes in order to avoid environmental concerns and the advantages that heterogeneous catalysis provides, we will develop the first SET heterogeneous catalysis with MOFs through the postsynthetic incorporation of chiral Ni or Ti-residues on the pore structure.

Publications

List of publications.
year	authors and title	journal	last update
2019	Javier Castells-Gil, Natalia M. Padial, Neyvis Almora-Barrios, Ivan da Silva, Diego Mateo, Josep Albero, Hermenegildo GarcÃa, Carlos MartÃ-Gastaldo De novo synthesis of mesoporous photoactive titanium( iv )â€“organic frameworks with MIL-100 topology published pages: 4313-4321, ISSN: 2041-6520, DOI: 10.1039/c8sc05218b	Chemical Science 10/15	2020-04-03
2019	Natalia M. Padial, Javier Castells-Gil, Neyvis Almora-Barrios, MarÃa Romero-Angel, IvÃ¡n da Silva, Mariam Barawi, Alba GarcÃa-SÃ¡nchez, VÃctor A. de la PeÃ±a Oâ€™Shea, Carlos MartÃ-Gastaldo Hydroxamate Titaniumâ€“Organic Frameworks and the Effect of Siderophore-Type Linkers over Their Photocatalytic Activity published pages: 13124-13133, ISSN: 0002-7863, DOI: 10.1021/jacs.9b04915	Journal of the American Chemical Society 141/33	2020-04-03
2019	Alejandro NuÃ±ezâ€Lopez, Marta Galbiati, Natalia M. Padial, Carolina R. Ganivet, Sergio Tatay, Emilio Pardo, Donatella Armentano, Carlos MartÃâ€Gastaldo Direct Visualization of Pyrrole Reactivity upon Confinement within a Cyclodextrin Metalâ€“Organic Framework published pages: 9179-9183, ISSN: 1433-7851, DOI: 10.1002/anie.201904890	Angewandte Chemie International Edition 58/27	2020-04-03
2019	Shengyang Ni, Natalia M. Padial, Cian Kingston, Julien C. Vantourout, Daniel C. Schmitt, Jacob T. Edwards, Monika M. Kruszyk, Rohan R. Merchant, Pavel K. Mykhailiuk, Brittany B. Sanchez, Shouliang Yang, Matthew A. Perry, Gary M. Gallego, James J. Mousseau, Michael R. Collins, Robert J. Cherney, Pavlo S. Lebed, Jason S. Chen, Tian Qin, Phil S. Baran A Radical Approach to Anionic Chemistry: Synthesis of Ketones, Alcohols, and Amines published pages: 6726-6739, ISSN: 0002-7863, DOI: 10.1021/jacs.9b02238	Journal of the American Chemical Society 141/16	2020-04-03
2020	Dongmin Xu, Nazaret Rivas-BascÃ³n, Natalia M. Padial, Kyle W. Knouse, Bin Zheng, Julien C. Vantourout, Michael A. Schmidt, Martin D. Eastgate, Phil S. Baran Enantiodivergent Formation of Câ€“P Bonds: Synthesis of P-Chiral Phosphines and Methylphosphonate Oligonucleotides published pages: 5785-5792, ISSN: 0002-7863, DOI: 10.1021/jacs.9b13898	Journal of the American Chemical Society 142/12	2020-04-03

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