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OLE-DIOX

Catalytic reductive carboxylation of unactivated olefins with carbon dioxide

Total Cost €

EC-Contrib. €

Partnership

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OLE-DIOX project word cloud

Explore the words cloud of the OLE-DIOX project. It provides you a very rough idea of what is the project "OLE-DIOX" about.

air dyes lengthy extensively plastics rubber recycling offers carboxylation reagents blocks opportunity source waste moisture ole operation components utmost protocol utilizes economically olefins pharmaceuticals building sensitive earth animal avoiding oil noble rely oxidation circular route textile contribution economy chemical expensive operates hydroformylation abundant event heavily materials protocols nor soaps unactivated manufacture mild acids chain hydrolysis technically c1 followed monoxide synthesis perfumes motifs toxic petroleum valuable nitriles industrially carboxylic industrial acid carbon feed rh detergents diox bulk techniques industry catalysts en dioxide unlike producing

Project "OLE-DIOX" data sheet

The following table provides information about the project.

Coordinator	FUNDACIO PRIVADA INSTITUT CATALA D'INVESTIGACIO QUIMICA Organization address address: AVENIDA PAISSOS CATALANS 16 city: TARRAGONA postcode: 43007 website: www.iciq.es contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.
Coordinator Country	Spain [ES]
Total cost	149˙500 €
EC max contribution	149˙500 € (100%)
Programme	1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
Code Call	ERC-2015-PoC
Funding Scheme	ERC-POC
Starting year	2016
Duration (year-month-day)	from 2016-06-01 to 2017-11-30

Partnership

Take a look of project's partnership.

#	participants	country	role	EC contrib. [€]
1	FUNDACIO PRIVADA INSTITUT CATALA D'INVESTIGACIO QUIMICA FUNDACIO PRIVADA INSTITUT CATALA D'INVESTIGACIO QUIMICA Organization address address: AVENIDA PAISSOS CATALANS 16 city: TARRAGONA postcode: 43007 website: www.iciq.es contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.	ES (TARRAGONA)	coordinator	149˙500.00

Map

Project objective

Carboxylic acids are building blocks of utmost importance in our chemical industry, as these motifs are extensively used in the manufacture of soaps, detergents, pharmaceuticals, rubber, plastics, dyes, textile, perfumes, and animal feed, among many others. Current industrial protocols for their synthesis rely heavily on toxic reagents, lengthy-step pathways or waste-producing procedures such as hydrolysis of nitriles or two-step techniques based on hydroformylation of olefins with highly toxic carbon monoxide with expensive noble catalysts (Rh) followed by oxidation. Unlike hydroformylation methods, OLE-DIOX offers the opportunity of promoting a carboxylation event using unactivated olefins, products produced in bulk from petroleum processing, with abundant carbon dioxide as C1 source. The protocol is user-friendly, with components that are neither air- nor moisture sensitive, utilizes earth-abundant catalysts and operates under mild conditions. OLE-DIOX represents an important contribution for our circular economy by effectively recycling bulk materials into valuable products in one-step operation. These unique features makes OLE-DIOX technically and economically viable for its implementation at large-scale en route to industrially-valuable carboxylic acids, thus avoiding lengthy and waste-producing protocols in the established oil-to-carboxylic acid process chain.

Publications

List of publications.
year	authors and title	journal	last update
2017	Morgane Gaydou, Toni Moragas, Francisco JuliÃ¡-HernÃ¡ndez, Ruben Martin Site-Selective Catalytic Carboxylation of Unsaturated Hydrocarbons with CO 2 and Water published pages: 12161-12164, ISSN: 0002-7863, DOI: 10.1021/jacs.7b07637	Journal of the American Chemical Society 139/35	2019-06-13
2017	Francisco JuliÃ¡-HernÃ¡ndez, Toni Moragas, Josep Cornella, Ruben Martin Remote carboxylation of halogenated aliphatic hydrocarbons with carbon dioxide published pages: 84-88, ISSN: 0028-0836, DOI: 10.1038/nature22316	Nature 545/7652	2019-06-13

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The information about "OLE-DIOX" are provided by the European Opendata Portal: CORDIS opendata.