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2D-CHEM SIGNED

Two-Dimensional Chemistry towards New Graphene Derivatives

Total Cost €

EC-Contrib. €

Partnership

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Outcomes and
results

2D-CHEM project word cloud

Explore the words cloud of the 2D-CHEM project. It provides you a very rough idea of what is the project "2D-CHEM" about.

perfluoropolyethylene derivatives perfluorinated forming organic prominent attempt materials date designed linking sustainable sheets chemistry textbook 2d enormously fluorographene functionalization behavior sensing envisage showed ev functionalized enhanced media explore dispersability hydrocarbon graphene 3d polar starting counterpart surprising rules synergistic blindly catalysis unreactive arising phenomena reg covalent suite limited inert hybrid molecules discipline graphenes covalently magnetic tentatively nanomaterials gained chemically preparing benefit band scaffold synthesis chemical opened suffer stable stands teflon inorganic joined experiments synthesized stability precursor grade few gap fluorescent imaging dimensional biomacromolecules indicates fg synthesizing

Project "2D-CHEM" data sheet

The following table provides information about the project.

Coordinator	UNIVERZITA PALACKEHO V OLOMOUCI Organization address address: KRIZKOVSKEHO 8 city: OLOMOUC postcode: 771 47 website: www.upol.cz contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.
Coordinator Country	Czech Republic [CZ]
Project website	http://www.2dchem.org
Total cost	1˙831˙102 €
EC max contribution	1˙831˙102 € (100%)
Programme	1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
Code Call	ERC-2015-CoG
Funding Scheme	ERC-COG
Starting year	2016
Duration (year-month-day)	from 2016-06-01 to 2021-05-31

Partnership

Take a look of project's partnership.

#	participants	country	role	EC contrib. [€]
1	UNIVERZITA PALACKEHO V OLOMOUCI UNIVERZITA PALACKEHO V OLOMOUCI Organization address address: KRIZKOVSKEHO 8 city: OLOMOUC postcode: 771 47 website: www.upol.cz contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.	CZ (OLOMOUC)	coordinator	1˙831˙102.00

Map

Project objective

The suite of graphene’s unique properties and applications can be enormously enhanced by its functionalization. As non-covalently functionalized graphenes do not target all graphene’s properties and may suffer from limited stability, covalent functionalization represents a promising way for controlling graphene’s properties. To date, only a few well-defined graphene derivatives have been introduced. Among them, fluorographene (FG) stands out as a prominent member because of its easy synthesis and high stability. Being a perfluorinated hydrocarbon, FG was believed to be as unreactive as the two-dimensional counterpart perfluoropolyethylene (Teflon®). However, our recent experiments showed that FG is not chemically inert and can be used as a viable precursor for synthesizing graphene derivatives. This surprising behavior indicates that common textbook grade knowledge cannot blindly be applied to the chemistry of 2D materials. Further, there might be specific rules behind the chemistry of 2D materials, forming a new chemical discipline we tentatively call 2D chemistry. The main aim of the project is to explore, identify and apply the rules of 2D chemistry starting from FG. Using the knowledge gained of 2D chemistry, we will attempt to control the chemistry of various 2D materials aimed at preparing stable graphene derivatives with designed properties, e.g., 1-3 eV band gap, fluorescent properties, sustainable magnetic ordering and dispersability in polar media. The new graphene derivatives will be applied in sensing, imaging, magnetic delivery and catalysis and new emerging applications arising from the synergistic phenomena are expected. We envisage that new applications will be opened up that benefit from the 2D scaffold and tailored properties of the synthesized derivatives. The derivatives will be used for the synthesis of 3D hybrid materials by covalent linking of the 2D sheets joined with other organic and inorganic molecules, nanomaterials or biomacromolecules.

Publications

List of publications.
year	authors and title	journal	last update
2019	Aristides Bakandritsos, Ravishankar G. Kadam, Pawan Kumar, Giorgio Zoppellaro, Miroslav Medved\', JiÅ™Ã TuÄek, Tiziano Montini, OndÅ™ej Tomanec, PavlÃna AndrÃ½skovÃ¡, Bohuslav DrahoÅ¡, Rajender S. Varma, Michal Otyepka, Manoj B. Gawande, Paolo Fornasiero, Radek ZboÅ™il Mixedâ€Valence Singleâ€Atom Catalyst Derived from Functionalized Graphene published pages: 1900323, ISSN: 0935-9648, DOI: 10.1002/adma.201900323	Advanced Materials 31/17	2019-08-29
2019	Aristides Bakandritsos, Petr Jakubec, Martin Pykal, Michal Otyepka Covalently functionalized graphene as a supercapacitor electrode material published pages: 25-33, ISSN: 2452-2627, DOI: 10.1016/j.flatc.2018.12.004	FlatChem 13	2019-08-29
2019	Hugo BarÃ¨s, Aristides Bakandritsos, Miroslav MedveÄ, Juri Ugolotti, Petr Jakubec, OndÅ™ej Tomanec, Sergii Kalytchuk, Radek ZboÅ™il, Michal Otyepka Bimodal role of fluorine atoms in fluorographene chemistry opens a simple way toward double functionalization of graphene published pages: 251-258, ISSN: 0008-6223, DOI: 10.1016/j.carbon.2019.01.059	Carbon 145	2019-08-29
2019	Eleni C. Vermisoglou, Petr Jakubec, Aristides Bakandritsos, Martin Pykal, Smita Talande, VojtÄ›ch Kupka, Radek ZboÅ™il, Michal Otyepka Chemical Tuning of Specific Capacitance in Functionalized Fluorographene published pages: 4698-4709, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.9b00655	Chemistry of Materials 31/13	2019-08-29
2018	Bruno de la Torre, Martin Å vec, Prokop Hapala, Jesus Redondo, OndÅ™ej KrejÄÃ, Rabindranath Lo, Debashree Manna, Amrit Sarmah, Dana NachtigallovÃ¡, JiÅ™Ã TuÄek, Piotr BÅ‚oÅ„ski, Michal Otyepka, Radek ZboÅ™il, Pavel Hobza, Pavel JelÃnek Non-covalent control of spin-state in metal-organic complex by positioning on N-doped graphene published pages: , ISSN: 2041-1723, DOI: 10.1038/s41467-018-05163-y	Nature Communications 9/1	2019-02-28
2018	Petr Lazar, Eva OtyepkovÃ¡, Martin Pykal, KlÃ¡ra ÄŒÃ©pe, Michal Otyepka Role of the puckered anisotropic surface in the surface and adsorption properties of black phosphorus published pages: 8979-8988, ISSN: 2040-3364, DOI: 10.1039/c8nr00329g	Nanoscale 10/19	2019-02-28
2018	Miroslav MedveÄ, Giorgio Zoppellaro, Juri Ugolotti, Dagmar MatochovÃ¡, Petr Lazar, TomÃ¡Å¡ PospÃÅ¡il, Aristides Bakandritsos, JiÅ™Ã TuÄek, Radek ZboÅ™il, Michal Otyepka Reactivity of fluorographene is triggered by point defects: beyond the perfect 2D world published pages: 4696-4707, ISSN: 2040-3364, DOI: 10.1039/c7nr09426d	Nanoscale 10/10	2019-02-28
2018	Dagmar MatochovÃ¡, Miroslav Medvedâ€™, Aristides Bakandritsos, TomÃ¡Å¡ SteklÃ½, Radek ZboÅ™il, Michal Otyepka 2D Chemistry: Chemical Control of Graphene Derivatization published pages: 3580-3585, ISSN: 1948-7185, DOI: 10.1021/acs.jpclett.8b01596	The Journal of Physical Chemistry Letters 9/13	2019-02-28
2018	Q Li, J P Froning, M Pykal, S Zhang, Z Wang, M VondrÃ¡k, P BanÃ¡Å¡, K ÄŒÃ©pe, P JureÄka, J Å poner, R ZboÅ™il, M Dong, M Otyepka RNA nanopatterning on graphene published pages: 31006, ISSN: 2053-1583, DOI: 10.1088/2053-1583/aabdf7	2D Materials 5/3	2019-02-28
2018	Aristides Bakandritsos, Demetrios D. Chronopoulos, Petr Jakubec, Martin Pykal, KlÃ¡ra ÄŒÃ©pe, Theodore Steriotis, Sergii Kalytchuk, Martin Petr, Radek ZboÅ™il, Michal Otyepka High-Performance Supercapacitors Based on a Zwitterionic Network of Covalently Functionalized Graphene with Iron Tetraaminophthalocyanine published pages: 1801111, ISSN: 1616-301X, DOI: 10.1002/adfm.201801111	Advanced Functional Materials 28/29	2019-02-28
2018	MarkÃ©ta PaloncÃ½ovÃ¡, Michal Langer, Michal Otyepka Structural Dynamics of Carbon Dots in Water and N , N -Dimethylformamide Probed by All-Atom Molecular Dynamics Simulations published pages: 2076-2083, ISSN: 1549-9618, DOI: 10.1021/acs.jctc.7b01149	Journal of Chemical Theory and Computation 14/4	2019-02-28
2019	Dario Mosconi, MatÃas Blanco, Teresa Gatti, Laura Calvillo, Michal Otyepka, Aristides Bakandritsos, Enzo Menna, Stefano Agnoli, Gaetano Granozzi Arene C H insertion catalyzed by ferrocene covalently heterogenized on graphene acid published pages: 318-328, ISSN: 0008-6223, DOI: 10.1016/j.carbon.2018.11.010	Carbon 143	2019-02-28
2019	Demetrios D. Chronopoulos, Miroslav Medvedâ€™, Piotr BÅ‚oÅ„ski, ZdenÄ›k NovÃ¡Äek, Petr Jakubec, OndÅ™ej Tomanec, Aristides Bakandritsos, Veronika NovotnÃ¡, Radek ZboÅ™il, Michal Otyepka Alkynylation of graphene via the Sonogashira Câ€“C cross-coupling reaction on fluorographene published pages: 1088-1091, ISSN: 1359-7345, DOI: 10.1039/c8cc08492k	Chemical Communications 55/8	2019-02-28

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