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DYNAPORE SIGNED

Dynamic responsive porous crystals

Total Cost €

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EC-Contrib. €

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Partnership

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 DYNAPORE project word cloud

Explore the words cloud of the DYNAPORE project. It provides you a very rough idea of what is the project "DYNAPORE" about.

controllably    structure    experimental    man    whilst    proof    catalysis    porous    relationship    integrates    dynamical    selectivity    controls    crystalline    blocked    reorganising    builds    sorption    solids    guide    mimics    characterisation    protein    multidisciplinary    made    diffraction    workflow    efficiency    organic    dynamic    composition    computation    function    demonstrated    reaction    functional    restructure    flexible    porosity    intended    harness    atomic    capability    chemical    structures    nature    discovery    optimise    methodology    perform    metal    linkers    synthesis    organisation    permits    evaluation    transferable    flexibility    guests    reagent    materials    maximises    transform    vision    rigid    dynamically    guest    dynamics    structural    create    environment    inhibition    cascade    inorganic    inspired    prediction    performance    property    synergic    road    frameworks    develops    computational    accelerate    chemistry    precision    classes    restructuring    separation    crystallinity   

Project "DYNAPORE" data sheet

The following table provides information about the project.

Coordinator
THE UNIVERSITY OF LIVERPOOL 

Organization address
address: BROWNLOW HILL 765 FOUNDATION BUILDING
city: LIVERPOOL
postcode: L69 7ZX
website: www.liverpool.ac.uk

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country United Kingdom [UK]
 Total cost 2˙493˙425 €
 EC max contribution 2˙493˙425 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2015-AdG
 Funding Scheme ERC-ADG
 Starting year 2016
 Duration (year-month-day) from 2016-10-01   to  2021-09-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    THE UNIVERSITY OF LIVERPOOL UK (LIVERPOOL) coordinator 2˙493˙425.00

Map

 Project objective

The project addresses the long-term vision of man-made materials with chemical selectivity and functional efficiency produced by dynamic structural flexibility. These materials are not intended as protein mimics; they are however inspired by nature’s use of flexible rather than rigid systems, with their ability to dynamically restructure around guests and thus perform highly specific chemistry. Such materials would transform chemical processes through their precision, for example by reorganising to accelerate each step of a cascade reaction without reagent or product inhibition. The road to this vision is blocked as we do not have the methodology and understanding to control such materials. The aim is to develop synergic, multidisciplinary experimental and computational capability to harness the dynamics of flexible crystalline porous solids for function, demonstrated in separation and catalysis. This will enable design and synthesis of materials that controllably adopt distinct structures according to their chemical environment to optimise performance. We will create a new workflow that integrates understanding of the structure-composition-dynamics-property relationship into the materials design and discovery process. This workflow builds on proof-of-concept in (i) chemical control of dynamical restructuring in flexible crystalline porous materials and in the use of dynamics to (ii) enhance function and (iii) guide synthesis. Crystalline flexible porous materials are selected because crystallinity maximises the atomic-scale understanding generated, which is transferable to other materials classes, whilst porosity permits sorption and organisation of guests that controls function. This inorganic materials chemistry project develops integrated capability in chemical synthesis (new metal-organic frameworks and linkers), computation (prediction and evaluation of structure and dynamical guest response), characterisation (e.g. by diffraction) and measurement of function.

 Publications

year authors and title journal last update
List of publications.
2019 Elliot J Carrington, Rémi Petuya, Rebecca K Hylton, Yong Yan, Dmytro Antypov, George Darling, Matthew Dyer, Neil G Berry, Alexandros P Katsoulidis, Matthew J Rosseinsky
A Highly Flexible Metal-Organic Framework Constructed from Asymmetric Flexible Linkers and Heptanuclear Zinc Carboxylate Secondary Building Units and its Anisotropic Dynamic Responses Exhibited During Guest Removal and Single Crystal Coordinated Solvent Exchange
published pages: , ISSN: 1528-7483, DOI: 10.26434/chemrxiv.8048321.v1
Crystal Growth & Design 2019-06-07
2019 Alexandros P. Katsoulidis, Dmytro Antypov, George F. S. Whitehead, Elliot J. Carrington, Dave J. Adams, Neil G. Berry, George R. Darling, Matthew S. Dyer, Matthew J. Rosseinsky
Chemical control of structure and guest uptake by a conformationally mobile porous material
published pages: 213-217, ISSN: 0028-0836, DOI: 10.1038/s41586-018-0820-9
Nature 565/7738 2019-06-06
2017 J. Haddad, G. F. S. Whitehead, A. P. Katsoulidis, M. J. Rosseinsky
In-MOFs based on amide functionalised flexible linkers
published pages: 327-335, ISSN: 1359-6640, DOI: 10.1039/c7fd00085e
Faraday Discussions 201 2019-06-06

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