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NANOCHEM SIGNED
Nanopores for New Molecular Nitrogen Chemistry
Total Cost €
0EC-Contrib. €
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0NANOCHEM project word cloud
Explore the words cloud of the NANOCHEM project. It provides you a very rough idea of what is the project "NANOCHEM" about.
characterisation
interactions
dynamic
clean
n2o4
n2h4
capture
fundamental
direct
scr
capacity
nanopores
nanoporous
environmentally
n2o
nox
captured
hybrid
no2
urea
adsorption
portable
relationships
molecular
extensive
porous
selective
decoration
loaded
improvement
construction
materials
mofs
functional
mitigation
structure
molecules
transport
storage
experiments
mild
host
medium
binding
reactor
relevance
substrates
society
reactivity
gain
functionalized
emphasis
function
stability
confined
structural
containing
industry
re
sustainable
situ
gas
efficient
catalytic
tests
release
framework
direction
nh3
static
synthesis
space
chemistry
stores
computational
pi
degradation
academia
pore
assembly
metal
spectroscopic
compounds
doped
environment
organic
energetic
catalysts
separation
hydrocarbons
impacts
denox
mof
substrate
energy
Project "NANOCHEM" data sheet
The following table provides information about the project.
| Coordinator |
THE UNIVERSITY OF MANCHESTER
Organization address contact info |
| Coordinator Country | United Kingdom [UK] |
| Total cost | 2˙498˙645 € |
| EC max contribution | 2˙498˙645 € (100%) |
| Programme |
1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC)) |
| Code Call | ERC-2016-ADG |
| Funding Scheme | ERC-ADG |
| Starting year | 2017 |
| Duration (year-month-day) | from 2017-06-01 to 2022-05-31 |
Partnership
Take a look of project's partnership.
| # | ||||
|---|---|---|---|---|
| 1 | THE UNIVERSITY OF MANCHESTER | UK (MANCHESTER) | coordinator | 2˙498˙645.00 |
Map
Project objective
We will study the adsorption, binding, transport and reactivity of N-containing substrates within the nanopores of functionalized and doped metal-organic framework (MOF) materials. A range of important target molecules (e.g., NH3, N2H4, N2O, NO, NO2 and N2O4) will be studied in this project, which aims to re-define the molecular chemistry for these energetic N-compounds in confined space, and to develop selective catalytic reduction (SCR) of NOx in the presence of NH3, urea and hydrocarbons. The PI has extensive experience in the field of coordination chemistry and hybrid materials, and seeks to change research direction to develop new gas phase catalysts and to gain fundamental understanding of molecular interactions, properties and function of specific energy, environmentally-related substrates within MOFs. Research objectives include the: • Design and synthesis of new porous MOFs with emphasis on the decoration of their pore environment and improvement of their structural stability and function; • Characterisation of host and substrate-loaded materials by state-of-the-art in situ structural, dynamic and spectroscopic methods for the construction of structure-function relationships, supported by computational analysis and modelling; • Adsorption, binding, release and separation of NH3, N2H4, N2O, NO, NO2 and N2O4 via both static and dynamic experiments; • Tests of degradation and selective catalytic reduction (SCR) of captured NOx molecules with NH3, urea and hydrocarbons under mild conditions using nanoporous MOFs as host catalysts; • Assembly of a MOF-based (i) catalytic deNOx reactor and (ii) NH3 storage system for potential portable applications. This project will deliver new functional materials as high capacity portable NH3 stores, efficient capture medium for NOx, and new catalysts for reduction and mitigation of NOx to deliver significant impacts to academia, industry and society of direct relevance to clean energy and sustainable environment.
Publications
| year | authors and title | journal | last update |
|---|---|---|---|
| 2019 |
Xinran Zhang, Ivan da Silva, Rodrigo Fazzi, Alena M. Sheveleva, Xue Han, Ben F. Spencer, Sergey A. Sapchenko, Floriana Tuna, Eric J. L. McInnes, Ming Li, Sihai Yang, Martin Schröder Iodine Adsorption in a Redox-Active Metal–Organic Framework: Electrical Conductivity Induced by Host−Guest Charge-Transfer published pages: 14145-14150, ISSN: 0020-1669, DOI: 10.1021/acs.inorgchem.9b02176 |
Inorganic Chemistry 58/20 | 2020-01-29 |
| 2019 |
Jiangnan Li, Xue Han, Xinran Zhang, Alena M. Sheveleva, Yongqiang Cheng, Floriana Tuna, Eric J. L. McInnes, Laura J. McCormick McPherson, Simon J. Teat, Luke L. Daemen, Anibal J. Ramirez-Cuesta, Martin Schröder, Sihai Yang Capture of nitrogen dioxide and conversion to nitric acid in a porous metal–organic framework published pages: 1085-1090, ISSN: 1755-4330, DOI: 10.1038/s41557-019-0356-0 |
Nature Chemistry 11/12 | 2020-01-29 |
| 2019 |
Xinchen Kang, Kai Lyu, Lili Li, Jiangnan Li, Louis Kimberley, Bin Wang, Lifei Liu, Yongqiang Cheng, Mark D. Frogley, Svemir Rudić, Anibal J. Ramirez-Cuesta, Robert A. W. Dryfe, Buxing Han, Sihai Yang, Martin Schröder Integration of mesopores and crystal defects in metal-organic frameworks via templated electrosynthesis published pages: , ISSN: 2041-1723, DOI: 10.1038/s41467-019-12268-5 |
Nature Communications 10/1 | 2020-01-29 |
| 2019 |
Gemma L. Smith, Jennifer E. Eyley, Xue Han, Xinran Zhang, Jiangnan Li, Nicholas M. Jacques, Harry G. W. Godfrey, Stephen P. Argent, Laura J. McCormick McPherson, Simon J. Teat, Yongqiang Cheng, Mark D. Frogley, Gianfelice Cinque, Sarah J. Day, Chiu C. Tang, Timothy L. Easun, Svemir Rudić, Anibal J. Ramirez-Cuesta, Sihai Yang, Martin Schröder Reversible coordinative binding and separation of sulfur dioxide in a robust metal–organic framework with open copper sites published pages: 1358-1365, ISSN: 1476-1122, DOI: 10.1038/s41563-019-0495-0 |
Nature Materials 18/12 | 2020-01-29 |
| 2019 |
Leo J. Small, Ryan C. Hill, James L. Krumhansl, Mara E. Schindelholz, Zhihengyu Chen, Karena W. Chapman, Xinran Zhang, Sihai Yang, Martin Schröder, Tina M. Nenoff Reversible MOF-Based Sensors for the Electrical Detection of Iodine Gas published pages: 27982-27988, ISSN: 1944-8244, DOI: 10.1021/acsami.9b09938 |
ACS Applied Materials & Interfaces 11/31 | 2020-01-29 |
| 2019 |
Harry G. W. Godfrey, Lydia Briggs, Xue Han, William J. F. Trenholme, Christopher G. Morris, Mathew Savage, Louis Kimberley, Oxana V. Magdysyuk, Michael Drakopoulos, Claire A. Murray, Chiu C. Tang, Mark D. Frogley, Gianfelice Cinque, Sihai Yang, Martin Schröder Analysis by synchrotron X-ray scattering of the kinetics of formation of an Fe-based metal-organic framework with high CO 2 adsorption published pages: 111104, ISSN: 2166-532X, DOI: 10.1063/1.5121644 |
APL Materials 7/11 | 2020-01-29 |
| 2019 |
Sergey A. Sapchenko, Marina O. Barsukova, Rodion V. Belosludov, Konstantin A. Kovalenko, Denis G. Samsonenko, Artem S. Poryvaev, Alena M. Sheveleva, Matvey V. Fedin, Artem S. Bogomyakov, Danil N. Dybtsev, Martin Schröder, Vladimir P. Fedin Understanding Hysteresis in Carbon Dioxide Sorption in Porous Metal–Organic Frameworks published pages: 6811-6820, ISSN: 0020-1669, DOI: 10.1021/acs.inorgchem.9b00016 |
Inorganic Chemistry 58/10 | 2020-01-29 |
| 2019 |
Xue Han, Sihai Yang, Martin Schröder Porous metal–organic frameworks as emerging sorbents for clean air published pages: 108-118, ISSN: 2397-3358, DOI: 10.1038/s41570-019-0073-7 |
Nature Reviews Chemistry 3/2 | 2020-01-29 |
| 2018 |
Zhenzhong Lu, Harry G. W. Godfrey, Ivan da Silva, Yongqiang Cheng, Mathew Savage, Pascal Manuel, Svemir Rudić, Anibal J. Ramirez-Cuesta, Sihai Yang, Martin Schröder Direct observation of supramolecular binding of light hydrocarbons in vanadium( iii ) and ( iv ) metal–organic framework materials published pages: 3401-3408, ISSN: 2041-6520, DOI: 10.1039/c8sc00330k |
Chemical Science 9/13 | 2019-02-28 |
| 2017 |
Vladimir V. Korolkov, Ivan G. Timokhin, Rolf Haubrichs, Emily F. Smith, Lixu Yang, Sihai Yang, Neil R. Champness, Martin Schröder, Peter H. Beton Supramolecular networks stabilise and functionalise black phosphorus published pages: , ISSN: 2041-1723, DOI: 10.1038/s41467-017-01797-6 |
Nature Communications 8/1 | 2019-02-28 |
| 2018 |
Thien D. Duong, Sergey A. Sapchenko, Ivan da Silva, Harry G. W. Godfrey, Yongqiang Cheng, Luke L. Daemen, Pascal Manuel, Anibal J. Ramirez-Cuesta, Sihai Yang, Martin Schröder Optimal Binding of Acetylene to a Nitro-Decorated Metal–Organic Framework published pages: 16006-16009, ISSN: 0002-7863, DOI: 10.1021/jacs.8b08504 |
Journal of the American Chemical Society 140/47 | 2019-02-28 |
| 2017 |
Adam D. Martin, Timothy L. Easun, Stephen P. Argent, William Lewis, Alexander J. Blake, Martin Schröder The effect of carboxylate position on the structure of a metal organic framework derived from cyclotriveratrylene published pages: 603-607, ISSN: 1466-8033, DOI: 10.1039/c6ce01965j |
CrystEngComm 19/4 | 2019-02-28 |
| 2018 |
Nicholas M. Jacques, Peter R. E. Rought, Detlev Fritsch, Mathew Savage, Harry G. W. Godfrey, Lei Li, Tamoghna Mitra, Mark D. Frogley, Gianfelice Cinque, Sihai Yang, Martin Schröder Locating the binding domains in a highly selective mixed matrix membrane via synchrotron IR microspectroscopy published pages: 2866-2869, ISSN: 1359-7345, DOI: 10.1039/c7cc08932e |
Chemical Communications 54/23 | 2019-02-28 |
| 2018 |
Tamoghna Mitra, Florian Moreau, Adam Nevin, Carlo U. Perotto, Alex Summerfield, E. Stephen Davies, Elizabeth A. Gibson, Timothy L. Easun, Martin Schröder Characterisation of redox states of metal–organic frameworks by growth on modified thin-film electrodes published pages: 6572-6579, ISSN: 2041-6520, DOI: 10.1039/c8sc00803e |
Chemical Science 9/31 | 2019-02-28 |
| 2017 |
Marina S. Zavakhina, Irina V. Yushina, Denis G. Samsonenko, Danil N. Dybtsev, Vladimir P. Fedin, Stephen P. Argent, Alexander J. Blake, Martin Schröder Halochromic coordination polymers based on a triarylmethane dye for reversible detection of acids published pages: 465-470, ISSN: 1477-9226, DOI: 10.1039/c6dt03969c |
Dalton Transactions 46/2 | 2019-02-20 |
| 2018 |
Yong Yan, Alice E. O’Connor, Gopikkaa Kanthasamy, George Atkinson, David R. Allan, Alexander J. Blake, Martin Schröder Unusual and Tunable Negative Linear Compressibility in the Metal–Organic Framework MFM-133(M) (M = Zr, Hf) published pages: 3952-3958, ISSN: 0002-7863, DOI: 10.1021/jacs.7b11747 |
Journal of the American Chemical Society 140/11 | 2019-02-28 |
| 2017 |
Yong Yan, Daniil I. Kolokolov, Ivan da Silva, Alexander G. Stepanov, Alexander J. Blake, Anne Dailly, Pascal Manuel, Chiu C. Tang, Sihai Yang, Martin Schröder Porous Metal–Organic Polyhedral Frameworks with Optimal Molecular Dynamics and Pore Geometry for Methane Storage published pages: 13349-13360, ISSN: 0002-7863, DOI: 10.1021/jacs.7b05453 |
Journal of the American Chemical Society 139/38 | 2019-02-28 |
| 2017 |
Aleksandr A. Sapianik, Ekaterina N. Zorina-Tikhonova, Mikhail A. Kiskin, Denis G. Samsonenko, Konstantin A. Kovalenko, Alexey A. Sidorov, Igor L. Eremenko, Danil N. Dybtsev, Alexander J. Blake, Stephen P. Argent, Martin Schröder, Vladimir P. Fedin Rational Synthesis and Investigation of Porous Metal–Organic Framework Materials from a Preorganized Heterometallic Carboxylate Building Block published pages: 1599-1608, ISSN: 0020-1669, DOI: 10.1021/acs.inorgchem.6b02713 |
Inorganic Chemistry 56/3 | 2019-02-28 |
| 2019 |
Peter Rought, Christopher Marsh, Simona Pili, Ian P. Silverwood, Victoria GarcÃa Sakai, Ming Li, Martyn S. Brown, Stephen P. Argent, Inigo Vitorica-Yrezabal, George Whitehead, Mark R. Warren, Sihai Yang, Martin Schröder Modulating proton diffusion and conductivity in metal–organic frameworks by incorporation of accessible free carboxylic acid groups published pages: , ISSN: 2041-6520, DOI: 10.1039/c8sc03022g |
Chemical Science | 2019-02-28 |
| 2018 |
Jian Lü, Cristina Perez-Krap, Fabien Trousselet, Yong Yan, Nada H. Alsmail, Bahar Karadeniz, Nicholas M. Jacques, William Lewis, Alexander J. Blake, François-Xavier Coudert, Rong Cao, Martin Schröder Polycatenated 2D Hydrogen-Bonded Binary Supramolecular Organic Frameworks (SOFs) with Enhanced Gas Adsorption and Selectivity published pages: 2555-2562, ISSN: 1528-7483, DOI: 10.1021/acs.cgd.8b00153 |
Crystal Growth & Design 18/4 | 2019-02-20 |
| 2017 |
Timothy L. Easun, Florian Moreau, Yong Yan, Sihai Yang, Martin Schröder Structural and dynamic studies of substrate binding in porous metal–organic frameworks published pages: 239-274, ISSN: 0306-0012, DOI: 10.1039/c6cs00603e |
Chemical Society Reviews 46/1 | 2019-02-28 |
| 2018 |
Vsevolod A. Bolotov, Konstantin A. Kovalenko, Denis G. Samsonenko, Xue Han, Xinran Zhang, Gemma L. Smith, Laura J. MCormick, Simon J. Teat, Sihai Yang, Matthew J. Lennox, Alice Henley, Elena Besley, Vladimir P. Fedin, Danil N. Dybtsev, Martin Schröder Enhancement of CO 2 Uptake and Selectivity in a Metal–Organic Framework by the Incorporation of Thiophene Functionality published pages: 5074-5082, ISSN: 0020-1669, DOI: 10.1021/acs.inorgchem.8b00138 |
Inorganic Chemistry 57/9 | 2019-02-28 |
| 2017 |
Andrea Laybourn, Juliano Katrib, Rebecca S. Ferrari-John, Christopher G. Morris, Sihai Yang, Ofonime Udoudo, Timothy L. Easun, Chris Dodds, Neil R. Champness, Samuel W. Kingman, Martin Schröder Metal–organic frameworks in seconds via selective microwave heating published pages: 7333-7338, ISSN: 2050-7488, DOI: 10.1039/c7ta01493g |
Journal of Materials Chemistry A 5/16 | 2019-02-28 |
| 2018 |
Joseph H. Carter, Xue Han, Florian Y. Moreau, Ivan da Silva, Adam Nevin, Harry G. W. Godfrey, Chiu C. Tang, Sihai Yang, Martin Schröder Exceptional Adsorption and Binding of Sulfur Dioxide in a Robust Zirconium-Based Metal–Organic Framework published pages: 15564-15567, ISSN: 0002-7863, DOI: 10.1021/jacs.8b08433 |
Journal of the American Chemical Society 140/46 | 2019-02-28 |
| 2017 |
Sergey A. Sapchenko, Pavel A. Demakov, Denis G. Samsonenko, Danil N. Dybtsev, Martin Schröder, Vladimir P. Fedin A Cryptand Metal-Organic Framework as a Platform for the Selective Uptake and Detection of Group I Metal Cations published pages: 2286-2289, ISSN: 0947-6539, DOI: 10.1002/chem.201605895 |
Chemistry - A European Journal 23/10 | 2019-02-28 |
| 2017 |
Xinran Zhang, Ivan da Silva, Harry G. W. Godfrey, Samantha K. Callear, Sergey A. Sapchenko, Yongqiang Cheng, Inigo Vitórica-Yrezábal, Mark D. Frogley, Gianfelice Cinque, Chiu C. Tang, Carlotta Giacobbe, Catherine Dejoie, Svemir Rudić, Anibal J. Ramirez-Cuesta, Melissa A. Denecke, Sihai Yang, Martin Schröder Confinement of Iodine Molecules into Triple-Helical Chains within Robust Metal–Organic Frameworks published pages: 16289-16296, ISSN: 0002-7863, DOI: 10.1021/jacs.7b08748 |
Journal of the American Chemical Society 139/45 | 2019-02-28 |
| 2017 |
Iñigo J. Vitórica-Yrezábal, Daniel Florin Sava, Grigore A. Timco, Martyn S. Brown, Mathew Savage, Harry G. W. Godfrey, Florian Moreau, Martin Schröder, Flor Siperstein, Lee Brammer, Sihai Yang, Martin P. Attfield, Joseph J. W. McDouall, Richard E. P. Winpenny Binding CO 2 by a Cr 8 Metallacrown published pages: 5527-5530, ISSN: 1433-7851, DOI: 10.1002/anie.201701726 |
Angewandte Chemie International Edition 56/20 | 2019-02-28 |
| 2018 |
Harry G. W. Godfrey, Ivan da Silva, Lydia Briggs, Joseph H. Carter, Christopher G. Morris, Mathew Savage, Timothy L. Easun, Pascal Manuel, Claire A. Murray, Chiu C. Tang, Mark D. Frogley, Gianfelice Cinque, Sihai Yang, Martin Schröder Ammonia Storage by Reversible Host-Guest Site Exchange in a Robust Metal-Organic Framework published pages: 14778-14781, ISSN: 1433-7851, DOI: 10.1002/anie.201808316 |
Angewandte Chemie International Edition 57/45 | 2019-02-28 |
| 2019 |
Lei Li, Ivan da Silva, Daniil I. Kolokolov, Xue Han, Jiangnan Li, Gemma Smith, Yongqiang Cheng, Luke L. Daemen, Christopher G. Morris, Harry G. W. Godfrey, Nicholas M. Jacques, Xinran Zhang, Pascal Manuel, Mark D. Frogley, Claire A. Murray, Anibal J. Ramirez-Cuesta, Gianfelice Cinque, Chiu C. Tang, Alexander G. Stepanov, Sihai Yang, Martin Schroder Post-synthetic modulation of the charge distribution in a metal–organic framework for optimal binding of carbon dioxide and sulfur dioxide published pages: , ISSN: 2041-6520, DOI: 10.1039/c8sc01959b |
Chemical Science | 2019-02-28 |
| 2019 |
Jack D. Humby, Oguarabau Benson, Gemma L. Smith, Stephen P. Argent, Ivan da Silva, Yongqiang Cheng, Svemir Rudić, Pascal Manuel, Mark D. Frogley, Gianfelice Cinque, Lucy K. Saunders, Iñigo J. Vitórica-Yrezábal, George F. S. Whitehead, Timothy L. Easun, William Lewis, Alexander J. Blake, Anibal J. Ramirez-Cuesta, Sihai Yang, Martin Schröder Host–guest selectivity in a series of isoreticular metal–organic frameworks: observation of acetylene-to-alkyne and carbon dioxide-to-amide interactions published pages: 1098-1106, ISSN: 2041-6520, DOI: 10.1039/c8sc03622e |
Chemical Science 10/4 | 2019-02-28 |
| 2016 |
Jamie A. Gould, Harprit Singh Athwal, Alexander J. Blake, William Lewis, Peter Hubberstey, Neil R. Champness, Martin Schröder Gas adsorption and structural diversity in a family of Cu(II) pyridyl-isophthalate metal–organic framework materials published pages: 20160334, ISSN: 1364-503X, DOI: 10.1098/rsta.2016.0334 |
Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences 375/2084 | 2019-02-28 |
| 2017 |
Christopher G. Morris, Nicholas M. Jacques, Harry G. W. Godfrey, Tamoghna Mitra, Detlev Fritsch, Zhenzhong Lu, Claire A. Murray, Jonathan Potter, Tom M. Cobb, Fajin Yuan, Chiu C. Tang, Sihai Yang, Martin Schröder Stepwise observation and quantification and mixed matrix membrane separation of CO 2 within a hydroxy-decorated porous host published pages: 3239-3248, ISSN: 2041-6520, DOI: 10.1039/c6sc04343g |
Chemical Science 8/4 | 2019-02-20 |
| 2018 |
Xue Han, Harry G. W. Godfrey, Lydia Briggs, Andrew J. Davies, Yongqiang Cheng, Luke L. Daemen, Alena M. Sheveleva, Floriana Tuna, Eric J. L. McInnes, Junliang Sun, Christina Drathen, Michael W. George, Anibal J. Ramirez-Cuesta, K. Mark Thomas, Sihai Yang, Martin Schröder Reversible adsorption of nitrogen dioxide within a robust porous metal–organic framework published pages: 691-696, ISSN: 1476-1122, DOI: 10.1038/s41563-018-0104-7 |
Nature Materials 17/8 | 2019-02-20 |
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