EDAX SIGNED
Beating Complexity through Selectivity: Excited state Dynamics from Anti-Stokes and non-linear resonant inelastic X-ray scattering
Total Cost €
0EC-Contrib. €
0Partnership
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Project "EDAX" data sheet
The following table provides information about the project.
| Coordinator |
UNIVERSITAET POTSDAM
Organization address contact info |
| Coordinator Country | Germany [DE] |
| Total cost | 2˙496˙250 € |
| EC max contribution | 2˙496˙250 € (100%) |
| Programme |
1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC)) |
| Code Call | ERC-2014-ADG |
| Funding Scheme | ERC-ADG |
| Starting year | 2016 |
| Duration (year-month-day) | from 2016-01-01 to 2020-12-31 |
Partnership
Take a look of project's partnership.
| # | ||||
|---|---|---|---|---|
| 1 | UNIVERSITAET POTSDAM | DE (POTSDAM) | coordinator | 1˙804˙565.00 |
| 2 | HELMHOLTZ-ZENTRUM BERLIN FUR MATERIALIEN UND ENERGIE GMBH | DE (BERLIN) | participant | 434˙750.00 |
| 3 | EUROPEAN X-RAY FREE-ELECTRON LASERFACILITY GMBH | DE (SCHENEFELD) | participant | 256˙935.00 |
Map
Project objective
The key to move from a mere description of static materials properties to the determination and control of functionality and chemistry lies in understanding dynamic pathways through multidimensional energy landscapes.
Through my efforts over the last decade my group accomplished breakthroughs towards the required excited states selectivity and to follow dynamic pathways with resonant inelastic soft x-ray scattering (RIXS) in three aspects: Non-linear RIXS for materials science to boost scattering efficiency. Time resolved and Anti-Stokes RIXS for back-ground free detection of excited states. Sub-natural line width RIXS to map out potential energy surfaces at selected atoms.
In the ERC research I link these unfolding fields and combine them with ab-initio treatment of excited states to create unprecedented back-ground free X-ray probes of excited states of matter and their dynamics. This will be femtosecond time resolved Anti-Stokes RIXS for excited state selectivity with transform limited pulses and doubly resonant soft X-ray 4 wave mixing to determine multi-center dynamics on atomic scales.
The ERC grant will answer long standing questions on the governing principles of functionality, regarding chemical pathways and energy landscapes in molecules as well as phase transitions, driven phases and emergence in functional materials.
These novel approaches become only now feasible through the unprecedented brilliance of Free-Electron Lasers and the efforts of my group over the last decade. The ERC grant will establish proof-of-principle at brilliant soft X-ray Free-Electron Lasers that will be followed by world leading, ideal conditions implemented at the European XFEL.
Publications
| year | authors and title | journal | last update |
|---|---|---|---|
| 2016 |
Kristjan Kunnus, Ida Josefsson, Ivan Rajkovic, Simon Schreck, Wilson Quevedo, Martin Beye, Sebastian Grübel, Mirko Scholz, Dennis Nordlund, Wenkai Zhang, Robert W Hartsock, Kelly J Gaffney, William F Schlotter, Joshua J Turner, Brian Kennedy, Franz Hennies, Simone Techert, Philippe Wernet, Michael Odelius, Alexander Föhlisch Anti-Stokes resonant x-ray Raman scattering for atom specific and excited state selective dynamics published pages: 103011, ISSN: 1367-2630, DOI: 10.1088/1367-2630/18/10/103011 |
New Journal of Physics 18/10 | 2019-09-02 |
| 2017 |
Danilo Kühn, Florian Sorgenfrei, Erika Giangrisostomi, Raphael Jay, Abdurrahman Musazay, Ruslan Ovsyannikov, Christian Stråhlman, Svante Svensson, Nils Mårtensson, Alexander Föhlisch Capabilities of Angle Resolved Time of Flight electron spectroscopy with the 60° wide angle acceptance lens published pages: , ISSN: 0368-2048, DOI: 10.1016/j.elspec.2017.06.008 |
Journal of Electron Spectroscopy and Related Phenomena | 2019-09-02 |
| 2017 |
Sebastian Eckert, Jesper Norell, Piter S. Miedema, Martin Beye, Mattis Fondell, Wilson Quevedo, Brian Kennedy, Markus Hantschmann, Annette Pietzsch, Benjamin E. Van Kuiken, Matthew Ross, Michael P. Minitti, Stefan P. Moeller, William F. Schlotter, Munira Khalil, Michael Odelius, Alexander Föhlisch Ultrafast Independent N−H and N−C Bond Deformation Investigated with Resonant Inelastic X-Ray Scattering published pages: 6088-6092, ISSN: 1433-7851, DOI: 10.1002/anie.201700239 |
Angewandte Chemie International Edition 56/22 | 2019-09-02 |
| 2016 |
S. Eckert, P.S. Miedema, W. Quevedo, B. O’Cinneide, M. Fondell, M. Beye, A. Pietzsch, M. Ross, M. Khalil, A. Föhlisch Molecular structures and protonation state of 2-Mercaptopyridine in aqueous solution published pages: 103-106, ISSN: 0009-2614, DOI: 10.1016/j.cplett.2016.01.050 |
Chemical Physics Letters 647 | 2019-09-02 |
| 2017 |
VinÃcius Vaz da Cruz, Emelie Ertan, Rafael C. Couto, Sebastian Eckert, Mattis Fondell, Marcus Dantz, Brian Kennedy, Thorsten Schmitt, Annette Pietzsch, Freddy F. Guimarães, Hans Ã…gren, Faris Gel\'mukhanov, Michael Odelius, Alexander Föhlisch, Victor Kimberg A study of the water molecule using frequency control over nuclear dynamics in resonant X-ray scattering published pages: 19573-19589, ISSN: 1463-9076, DOI: 10.1039/C7CP01215B |
Phys. Chem. Chem. Phys. 19/30 | 2019-09-02 |
| 2016 |
Daniel Schick, Sebastian Eckert, Niko Pontius, Rolf Mitzner, Alexander Föhlisch, Karsten Holldack, Florian Sorgenfrei Versatile soft X-ray-optical cross-correlator for ultrafast applications published pages: 54304, ISSN: 2329-7778, DOI: 10.1063/1.4964296 |
Structural Dynamics 3/5 | 2019-09-02 |
| 2017 |
Sebastian Eckert, Jesper Norell, Piter S. Miedema, Martin Beye, Mattis Fondell, Wilson Quevedo, Brian Kennedy, Markus Hantschmann, Annette Pietzsch, Benjamin E. Van Kuiken, Matthew Ross, Michael P. Minitti, Stefan P. Moeller, William F. Schlotter, Munira Khalil, Michael Odelius, Alexander Föhlisch Untersuchung unabhängiger N-H- und N-C-Bindungsverformungen auf ultrakurzen Zeitskalen mit resonanter inelastischer Röntgenstreuung published pages: 6184-6188, ISSN: 0044-8249, DOI: 10.1002/ange.201700239 |
Angewandte Chemie 129/22 | 2019-09-02 |
| 2018 |
Jesper Norell, Raphael M. Jay, Markus Hantschmann, Sebastian Eckert, Meiyuan Guo, Kelly J. Gaffney, Philippe Wernet, Marcus Lundberg, Alexander Föhlisch, Michael Odelius Fingerprints of electronic, spin and structural dynamics from resonant inelastic soft X-ray scattering in transient photo-chemical species published pages: 7243-7253, ISSN: 1463-9076, DOI: 10.1039/c7cp08326b |
Physical Chemistry Chemical Physics 20/10 | 2019-09-02 |
| 2017 |
Mattis Fondell, Sebastian Eckert, Raphael M. Jay, Christian Weniger, Wilson Quevedo, Johannes Niskanen, Brian Kennedy, Florian Sorgenfrei, Daniel Schick, Erika Giangrisostomi, Ruslan Ovsyannikov, Katrin Adamczyk, Nils Huse, Philippe Wernet, Rolf Mitzner, Alexander Föhlisch Time-resolved soft X-ray absorption spectroscopy in transmission mode on liquids at MHz repetition rates published pages: 54902, ISSN: 2329-7778, DOI: 10.1063/1.4993755 |
Structural Dynamics 4/5 | 2019-09-02 |
| 2017 |
Rafael C. Couto, VinÃcius V. Cruz, Emelie Ertan, Sebastian Eckert, Mattis Fondell, Marcus Dantz, Brian Kennedy, Thorsten Schmitt, Annette Pietzsch, Freddy F. Guimarães, Hans Ã…gren, Faris Gel’mukhanov, Michael Odelius, Victor Kimberg, Alexander Föhlisch Selective gating to vibrational modes through resonant X-ray scattering published pages: 14165, ISSN: 2041-1723, DOI: 10.1038/ncomms14165 |
Nature Communications 8 | 2019-09-02 |
| 2017 |
Annette Pietzsch, Alexander Föhlisch Local Maps of Potential Energy Surfaces and Chemical Pathways published pages: 8-13, ISSN: 0894-0886, DOI: 10.1080/08940886.2017.1289799 |
Synchrotron Radiation News 30/2 | 2019-09-02 |
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